- Was the oldest son of actor Joseph Jefferson and the brother of actors William Jefferson, Joseph Jefferson Jr. and Thomas Jefferson.
- Was his father's business manager.
- Was named after his father's half brother, actor and comedian Charles Burke, who died in 1854.
- He would often join his father on fishing trips with former President Grover Cleveland.
- His wife, Edna Carey was a member of the "Rip Van Winkle" cast that starred his father.
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